Magnetic ordering and excitations of Cu₂Te₂O₅Cl₂ are analyzed in terms of a tetramerized spin model for the tetrahedral Cu clusters of spin 1/2. The mean-field model is able to account for the main properties of the incommensurable magnetic structure observed by Zaharko et al. [Phys. Rev. B 73, 064422 (2006)]. The calculated excitation spectra show many similarities with the experimental neutron-scattering results. Close to a magnetic Bragg point at 2 K, the theory predicts the presence of a quasielastic phason mode and an inelastic amplitude mode at about 0.6 meV. This is in qualitative agreement with experimental observations of Prša et al., but the amplitude mode is observed at the much higher energy of about 2.5 meV. This discrepancy is puzzling since the tetrahedral Cu-spin system, in any other respect, behaves as a system of large local spins coupled with each other in a three-dimensional fashion. Preliminary model calculations for the Cu₂Te₂O₅Br₂ system lead to the same conclusion.
Udgivelsesdato: 7. Januar