Magnetic ordering and spin excitations in Mn(dca)2(pyz) [dca = N (CN)2-, pyz = pyrazine]

Research output: Contribution to journal › Journal article › Research › peer-review

Standard

Magnetic ordering and spin excitations in Mn(dca)2(pyz) [dca = N (CN)2-, pyz = pyrazine]. / Manson, J. L.; Bordallo, H. N.; Lynn, J. W.; Huang, Q.; Feyerherm, R.; Loose, A.; Chapon, L.; Argyriou, D. N.

In: Applied Physics A, Vol. 74, No. SUPPL.I, 01.12.2002, p. 722-724.

Research output: Contribution to journal › Journal article › Research › peer-review

Harvard

Manson, JL, Bordallo, HN, Lynn, JW, Huang, Q, Feyerherm, R, Loose, A, Chapon, L & Argyriou, DN 2002, 'Magnetic ordering and spin excitations in Mn(dca)2(pyz) [dca = N (CN)2-, pyz = pyrazine]', Applied Physics A, vol. 74, no. SUPPL.I, pp. 722-724. https://doi.org/10.1007/s003390201662

APA

Manson, J. L., Bordallo, H. N., Lynn, J. W., Huang, Q., Feyerherm, R., Loose, A., Chapon, L., & Argyriou, D. N. (2002). Magnetic ordering and spin excitations in Mn(dca)2(pyz) [dca = N (CN)2-, pyz = pyrazine]. Applied Physics A, 74(SUPPL.I), 722-724. https://doi.org/10.1007/s003390201662

Vancouver

Manson JL, Bordallo HN, Lynn JW, Huang Q, Feyerherm R, Loose A et al. Magnetic ordering and spin excitations in Mn(dca)2(pyz) [dca = N (CN)2-, pyz = pyrazine]. Applied Physics A. 2002 Dec 1;74(SUPPL.I):722-724. https://doi.org/10.1007/s003390201662

Author

Manson, J. L. ; Bordallo, H. N. ; Lynn, J. W. ; Huang, Q. ; Feyerherm, R. ; Loose, A. ; Chapon, L. ; Argyriou, D. N. / Magnetic ordering and spin excitations in Mn(dca)2(pyz) [dca = N (CN)2-, pyz = pyrazine]. In: Applied Physics A. 2002 ; Vol. 74, No. SUPPL.I. pp. 722-724.

Bibtex

@article{a9cdcefa62d545a2bfa03575b176a720,
title = "Magnetic ordering and spin excitations in Mn(dca)2(pyz) [dca = N (CN)2-, pyz = pyrazine]",
abstract = "We have studied the T- and H-dependent magnetism in Mn(dca)2(pyz) [dca = N(CN)2-, pyz = pyrazine] using neutron-scattering methods. The crystal structure can be viewed as a molecular analog of ReO3, where 1D Mn-pyz-Mn chains connect 2D Mn(dca)2 square sheets to form a 3D network. In zero field, the Mn2+ moments order antiferromagnetically below 2.53(2) K along the ac diagonal with a magnitude of 4.15(6)μB at 1.35 K. The field-dependent response of the [111] magnetic reflection is consistent with spin-flop and induced ferromagnetic phase transitions as previously observed in magnetization measurements. Diffuse-scattering studies indicated no evidence for low-dimensional spin correlations. Using quasielastic neutron scattering, a low-energy spin-wave excitation was observed at ∼0.23 meV, which is ∼1/6 the momentum transfer observed in Mn(dca)2 owing to a reduced number of magnetic nearest neighbors.",
author = "Manson, {J. L.} and Bordallo, {H. N.} and Lynn, {J. W.} and Q. Huang and R. Feyerherm and A. Loose and L. Chapon and Argyriou, {D. N.}",
year = "2002",
month = dec,
day = "1",
doi = "10.1007/s003390201662",
language = "English",
volume = "74",
pages = "722--724",
journal = "Applied Physics A: Materials Science & Processing",
issn = "0947-8396",
publisher = "Springer",
number = "SUPPL.I",

}

RIS

TY - JOUR

T1 - Magnetic ordering and spin excitations in Mn(dca)2(pyz) [dca = N (CN)2-, pyz = pyrazine]

AU - Manson, J. L.

AU - Bordallo, H. N.

AU - Lynn, J. W.

AU - Huang, Q.

AU - Feyerherm, R.

AU - Loose, A.

AU - Chapon, L.

AU - Argyriou, D. N.

PY - 2002/12/1

Y1 - 2002/12/1

N2 - We have studied the T- and H-dependent magnetism in Mn(dca)2(pyz) [dca = N(CN)2-, pyz = pyrazine] using neutron-scattering methods. The crystal structure can be viewed as a molecular analog of ReO3, where 1D Mn-pyz-Mn chains connect 2D Mn(dca)2 square sheets to form a 3D network. In zero field, the Mn2+ moments order antiferromagnetically below 2.53(2) K along the ac diagonal with a magnitude of 4.15(6)μB at 1.35 K. The field-dependent response of the [111] magnetic reflection is consistent with spin-flop and induced ferromagnetic phase transitions as previously observed in magnetization measurements. Diffuse-scattering studies indicated no evidence for low-dimensional spin correlations. Using quasielastic neutron scattering, a low-energy spin-wave excitation was observed at ∼0.23 meV, which is ∼1/6 the momentum transfer observed in Mn(dca)2 owing to a reduced number of magnetic nearest neighbors.

AB - We have studied the T- and H-dependent magnetism in Mn(dca)2(pyz) [dca = N(CN)2-, pyz = pyrazine] using neutron-scattering methods. The crystal structure can be viewed as a molecular analog of ReO3, where 1D Mn-pyz-Mn chains connect 2D Mn(dca)2 square sheets to form a 3D network. In zero field, the Mn2+ moments order antiferromagnetically below 2.53(2) K along the ac diagonal with a magnitude of 4.15(6)μB at 1.35 K. The field-dependent response of the [111] magnetic reflection is consistent with spin-flop and induced ferromagnetic phase transitions as previously observed in magnetization measurements. Diffuse-scattering studies indicated no evidence for low-dimensional spin correlations. Using quasielastic neutron scattering, a low-energy spin-wave excitation was observed at ∼0.23 meV, which is ∼1/6 the momentum transfer observed in Mn(dca)2 owing to a reduced number of magnetic nearest neighbors.

UR - http://www.scopus.com/inward/record.url?scp=0347297381&partnerID=8YFLogxK

U2 - 10.1007/s003390201662

DO - 10.1007/s003390201662

M3 - Journal article

AN - SCOPUS:0347297381

VL - 74

SP - 722

EP - 724

JO - Applied Physics A: Materials Science & Processing

JF - Applied Physics A: Materials Science & Processing

SN - 0947-8396

IS - SUPPL.I

ER -

ID: 203940247