Coherence Time Extension by Large-Scale Optical Spin Polarization in a Rare-Earth Doped Crystal
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Coherence Time Extension by Large-Scale Optical Spin Polarization in a Rare-Earth Doped Crystal. / Welinski, Sacha; Tiranov, Alexey; Businger, Moritz; Ferrier, Alban; Afzelius, Mikael; Goldner, Philippe.
In: Physical Review X, Vol. 10, No. 3, 031060, 16.09.2020.Research output: Contribution to journal › Journal article › Research › peer-review
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TY - JOUR
T1 - Coherence Time Extension by Large-Scale Optical Spin Polarization in a Rare-Earth Doped Crystal
AU - Welinski, Sacha
AU - Tiranov, Alexey
AU - Businger, Moritz
AU - Ferrier, Alban
AU - Afzelius, Mikael
AU - Goldner, Philippe
PY - 2020/9/16
Y1 - 2020/9/16
N2 - Optically addressable spins are actively investigated in quantum communication, processing, and sensing. Optical and spin coherence lifetimes, which determine quantum operation fidelity and storage time, are often limited by spin-spin interactions, which can be decreased by polarizing spins. Spin polarization can be achieved using optical pumping, large magnetic fields, or mK-range temperatures. Here, we show that optical pumping of a small fraction of ions with a fixed-frequency laser, coupled with spin-spin interactions and spin diffusion, leads to substantial spin polarization in a paramagnetic rare-earth doped crystal, Yb-171(3+): Y2SiO5. Indeed, more than 90% spin polarization has been achieved at 2 K and zero magnetic field. Using this spin polarization mechanism, we further demonstrate an increase in optical coherence lifetime from 0.3 ms to 0.8 ms, due to a strong decrease in spin-spin interactions. This effect opens the way to new schemes for obtaining long optical and spin coherence lifetimes in various solid-state systems such as ensembles of rare-earth ions or color centers in diamond, which are of interest for a broad range of quantum technologies.
AB - Optically addressable spins are actively investigated in quantum communication, processing, and sensing. Optical and spin coherence lifetimes, which determine quantum operation fidelity and storage time, are often limited by spin-spin interactions, which can be decreased by polarizing spins. Spin polarization can be achieved using optical pumping, large magnetic fields, or mK-range temperatures. Here, we show that optical pumping of a small fraction of ions with a fixed-frequency laser, coupled with spin-spin interactions and spin diffusion, leads to substantial spin polarization in a paramagnetic rare-earth doped crystal, Yb-171(3+): Y2SiO5. Indeed, more than 90% spin polarization has been achieved at 2 K and zero magnetic field. Using this spin polarization mechanism, we further demonstrate an increase in optical coherence lifetime from 0.3 ms to 0.8 ms, due to a strong decrease in spin-spin interactions. This effect opens the way to new schemes for obtaining long optical and spin coherence lifetimes in various solid-state systems such as ensembles of rare-earth ions or color centers in diamond, which are of interest for a broad range of quantum technologies.
KW - QUANTUM MEMORY
KW - TRANSITIONS
KW - STORAGE
U2 - 10.1103/PhysRevX.10.031060
DO - 10.1103/PhysRevX.10.031060
M3 - Journal article
VL - 10
JO - Physical Review X
JF - Physical Review X
SN - 2160-3308
IS - 3
M1 - 031060
ER -
ID: 249163497